FACULTY OF PHYSICS & ENGINEERING PHYSICS

DEPARTMENT OF NUCLEAR PHYSICS - NUCLEAR ENGINEERING - MEDICAL PHYSICS

Combination of experimental and simulation methods for determination of effective atomic number by Rayleigh-Compton scattering technique

Le Hoang Minh, Van Thi Thu Trang, Tran Thien Thanh

JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY 2025

Abstract:

This paper presents the gamma scattering technique to determine substance' component concentrations. The experimental and simulated R/C ratios of binary oxide samples (Fe2O3and SiO2) were measured. The concentration ​​of each element were interpolated, with a bias relative less than 5% for the elements in the reference samples. The elements' experimental and theoretical Rayleigh-Compton ratio values had a robust relationship in the equation RexpR/C=1.03×RtheoR/C (n = 11; r = 0.99; p-value < 0.01). The Zeff interpolation results and the calculation results from the theoretical formulas have good agreement with an average difference of 5%.

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Trần Thiện Thanh, Văn Tấn Phát, Lê Hoàng Minh, Huỳnh Đình Chương, Võ Hoàng Nguyên, Nguyễn Trí Toàn Phúc, Lê Quang Vương, Nguyễn Duy Thông, Châu Văn Tạo
 
Sci. Tech. Dev. J. - Nat. Sci.; 4(2):Online-First
 
TÓM TẮT: 
Các thông số đặc trưng của vật liệu liên quan đến tương tác của bức xạ photon như: hệ số suy giảm khối, số nguyên tử hiệu dụng, mật độ electron là những dữ liệu cần thiết được yêu cầu trong nhiều công việc như chẩn đoán và xạ trị ung thư, chiếu xạ công nghiệp, tính liều lượng bức xạ, che chắn phóng xạ, phân tích hàm lượng nguyên tố và đồng vị phóng xạ. Trong bài báo này, các mô hình lý thuyết như tham số dạng phi tương đối tính (NRFF), tham số dạng tương đối tính (RFF), tham số dạng hiệu chỉnh (MFF) được sử dụng để tính toán tỉ số Rayleigh-Compton đối với các nguyên tố có 6<=Z<=82 tại năng lượng 59,5 keV. Kết quả chỉ ra rằng có sự khác biệt lớn giữa các mô hình tính toán đối với bia có số nguyên tử lớn. Giá trị trung bình của tỉ số Rayleigh-Compton theo số nguyên tử Z được làm khớp hàm bậc hai mô tả khá tốt quy luật phụ thuộc này với hệ số tương quan R2 =0,996. Bên cạnh đó, hệ đo thực nghiệm cũng được thiết kế và thực nghiệm đo đạc đối với một số bia như nhôm, đồng và chì tại góc tán xạ 150o sử dụng nguồn 241Am bằng đầu dò Si(Li) để kiểm chứng với kết quả tính toán lý thuyết. Kết quả thực nghiệm ban đầu đã chỉ ra rằng có sự phù hợp tốt giữa các mô hình lý thuyết với các bia nhôm, đồng và chì với độ sai biệt dưới 20%. Trong tương lai, chúng tôi sẽ tiến hành thực nghiệm với nhiều dạng bia khác nhau để đánh giá chi tiết hơn.
Từ khoá: NRFF, RFF, MFF, Tỉ số Rayleigh-Compton, đầu dò Si(Li)
 
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Bulk density determination of concrete by gamma-ray transmission using a 137Cs source and NaI(Tl) spectrometry: MCNP-based calibration and experimental validation across varying aggregate compositions

Huynh Dinh Chuong, Van Thi Thu Trang, Vo Hoang Nguyen, Le Thi Ngoc Trang, Nguyen Thi Truc Linh, Tran Thien Thanh

Radiation Physics and Chemistry, Vol 248(2026),114145

Abstract:

This paper presents a gamma-ray transmission method for the non-destructive determination of concrete bulk density. The experimental setup comprises a137Cs source, a NaI(Tl) detector, and lead collimators arranged in a narrow-beam transmission geometry. An MCNP model was developed to closely replicate the measurement configuration and was subsequently used to generate pulse-height spectra for elemental and concrete specimens covering densities of 2.10 – 8.96 g cm−3 and thicknesses of 1 – 15 cm. From each spectrum, the net area of the 661.7 keV peak was extracted, and the attenuation indicator R was defined as the ratio of the peak areas recorded with and without the specimen. The simulations were benchmarked against measurements for aluminum and copper reference specimens at different thicknesses, showing good agreement in spectral response and relative deviations between simulated and experimental R values below 0.8%. Using the simulated R dataset, a linear calibration curve was established, enabling concrete bulk density to be determined without prior knowledge of the elemental composition. The method was applied to 22 concrete specimens fabricated with different aggregate systems, including ordinary concretes and concretes incorporating heavyweight additives (e.g., barite, Bi2O3, Fe2O3, and steel chips). These specimens covered densities of 2.2 – 2.6 g cm−3 and thicknesses of 3 – 15 cm. Each specimen was measured at nine locations to assess spatial variability, and the weighted mean was taken as the representative bulk density. The resulting densities agree well with reference values obtained from mass-to-volume measurements, with relative deviations not exceeding 3.74% for all specimens. A coverage-probability–based statistical framework, augmented by additional sampling, was introduced to assess and improve measurement reliability when structural heterogeneity produces spatial variations in the inferred density. These preliminary results demonstrate that the proposed method is reliable and well suited for rapid concrete quality control.

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Nguyen Anh TUAN and Chau Van TAO

Nuclear Technology & Radiation Protection: Year 2020, Vol. 35, No. 1, pp. 36-41

Abstract:

An electron beam from the UELR-10-15S2 accelerator (average energy of 9.92 ± 0.48 MeV) was applied to irradiate food and medical items at the Research and Development Center for Radiation Technology, Vietnam Atomic Energy Institute, Vietnam. The materials are under an electron beam window, such as irradiation products, conveyor, magnet and shielding mate- rial for the magnet coil, bombarded by electrons and generated X-ray (bremsstrahlung effect). In this article, X-ray conversion efficiency from polypropylene, aluminum, iron, and lead bombarded by an electron beam from the UELR-10-15S2 accelerator is measured by the film dosimeter and simulated by the MCNP4c2 code, and there is good agreement between the calculation and measurement results. The results show that X-ray conversion efficiency is the highest from lead (4.3 %), so the gamma - neutron reaction (Q-value of –6.74 MeV for 207Pb) has to be studied in food and medical items irradiated by a 10 MeV eelectron beam.

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Nguyen Huu Quyet, Le Hong Khiem, Trinh Thi Thu My, Nguyen Thi Bao My, Marina Frontasieva, Inga Zinicovscaia, Nguyen An Son, Tran Thien Thanh, Le Dai Nam, Khuat Thi Hong, Nguyen Ngoc Mai, Trinh Dinh Trung, Duong Van Thang, Nguyen Thi Thuy Hang

Environmental Engineering and Management Journal

Abstract:

Atmospheric deposition of chemical elements in the Hanoi region has been investigated in this study based on moss biomonitoring. Twenty-seven Barbula indica moss samples were collected from the end of 2016 to the beginning of 2017, and the concentrations of 33 chemical elements in the samples were determined by instrumental neutron activation analysis. The results show that Hanoi’s air is highly polluted with Zn, Ba and Ta, and slightly polluted with Al, Cl, Sc, Ti, V, Cr, Mn, Fe, Ni, Co, As, Cd, Sb, La, Ce, Sm, Gd, Tb, Yb, Hf, Th and U. A determination of the possible pollution sources has been made for the analyzed elements; namely: coal and oil combustion are the main sources of V, Ni, Co and As; vehicle exhaust and non-exhaust sources, as well as industrial emissions, are the main sources of Mn, Co, Cd and Ba; construction dust is the source of Ca, Mg and Sb; various industries are the sources of Cr and Ni; the dust from cement kilns and ash from biomass burning is responsible for K and Cl; two-stroke motor vehicles, galvanizing factories and tire wear are the sources of Zn; and Br may be emitted from burning wastes.

 

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Benchmarking PHITS for radiation dose assessment from fly ash-blended concrete using MCNP6 and ResRad-Build

Lam Duy Nhat, Le Huu Loi, Le Quang Vuong, Vu Tuan Minh, Ho Van Doanh, Phan Long Ho, Tran Thien Thanh, Hoang Duc Tam

Applied Radiation and Isotopes, vol. 234, p. 112658, Apr. 2026

Abstract

In this study, the PHITS Monte Carlo code is applied for the first time to evaluate indoor radiation exposure associated with fly ash–blended concrete, and its performance is systematically benchmarked against the widely used ResRad-Build program and MCNP6 code. A reference room conforming to RP-112 dimensions (5 m × 4 m × 2.8 m) was modeled, and eight concrete mixtures containing 0–50% fly ash were investigated. The activity concentrations of 226Ra, 232Th, and 40K, along with material composition ratios and densities, were used as input parameters for simulations with PHITS, ResRad-Build, and MCNP6. The annual effective doses calculated using PHITS ranged from 0.378 to 0.489 mSv.y−1. The maximum relative deviations between PHITS and MCNP6 and between PHITS and ResRad-Build were 5.9% and 7.9%, respectively. PHITS exhibited the closest agreement with the reference dose estimate derived from measured activity concentrations, with a maximum relative deviation of 3.6%. These findings clearly demonstrate that PHITS is a highly reliable and effective tool for assessing indoor radiation exposure from building materials.

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